Peking University, Nov. 16, 2015: Most parent compounds of iron-based high temperature superconductors display a finite temperature “nematic” phase transition with spontaneous breaking of the 4-fold crystal rotation symmetry. This transition is usually accompanied by a stripe antiferromagnetic ordering transition at the same or slightly lower temperature. For this reason the driving force of nematicity in these iron-based materials is usually regarded as the antiferromagnetic correlation.
FeSe however shows very different phenomenology. It has a nematic phase transition at 90Kelvin but no magnetic order down to the lowest temperature. And recent nuclear magnetic resonance studies do not see enhancement of low energy spin fluctuation across the nematic transition in FeSe. People thus speculate that the nematic transition in FeSe is not driven by magnetic correlation but possibly orbital order.
Prof. Wang Fa of ICQM at Peking University, in collaboration with Prof. Kivelson of Stanford University and Prof. Dung-Hai Lee of UC Berkeley, challenged this perception of non-magnetic mechanism for nematicity in FeSe. They established by theoretical arguments and numerical results that a “nematic quantum paramagnet” phase can exist for frustrated spin-1 models on square lattice. This phase spontaneously breaks 4-fold crystal rotation symmetry but has no magnetic order and no low-energy spin excitations. They argued that the nematic quantum paramagnet phase can explain the unusual phase diagram of FeSe, and predicted the existence of finite energy spin fluctuations at both stripe and Neel ordering wavevectors. This work has been published in Nature Physics [Nature Physics 11, 959 (2015)].
The work done in PKU was supported by the National Science Foundation of China(Grant No. 11374018) andNational Key Basic Research Program of China (Grant No. 2014CB920902), and the “Thousand Talents Program for Distinguished Young Scholars”.
Left: Schematic depiction of two prototypical wavefunctions of nematic quantum paramagnet states. The spin-1 moments on solid blue lines form AKLT chains. Right: Spin excitation gap(S="1)" and spin-singlet excitation gap(S="0)" for 4x4 square lattice J1-J2 Heisenberg model. Around J2/J1="0.6" the spin gap is large but the spin-singlet gap is very small, suggesting nematic quantum paramagnet ground states in the thermodynamic limit.
Edited by: Zhang Jiang
Source: School of Physics
Left: Schematic depiction of two prototypical wavefunctions of nematic quantum paramagnet states. The spin-1 moments on solid blue lines form AKLT chains. Right: Spin excitation gap(S="1)" and spin-singlet excitation gap(S="0)" for 4x4 square lattice J1-J2 Heisenberg model. Around J2/J1="0.6" the spin gap is large but the spin-singlet gap is very small, suggesting nematic quantum paramagnet ground states in the thermodynamic limit.
